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CN112479282A - Efficient composite desulfurization wastewater treatment agent and preparation method thereof - Google Patents

Efficient composite desulfurization wastewater treatment agent and preparation method thereof Download PDF

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Publication number
CN112479282A
CN112479282A CN202011393993.5A CN202011393993A CN112479282A CN 112479282 A CN112479282 A CN 112479282A CN 202011393993 A CN202011393993 A CN 202011393993A CN 112479282 A CN112479282 A CN 112479282A
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desulfurization wastewater
wastewater treatment
treatment agent
parts
mass
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裴迪
王斌
汤友志
陈艳
李圣轶
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Beijing Guangyao Environmental Engineering Co ltd
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Beijing Guangyao Environmental Engineering Co ltd
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    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/28Treatment of water, waste water, or sewage by sorption
    • C02F1/281Treatment of water, waste water, or sewage by sorption using inorganic sorbents
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/28Treatment of water, waste water, or sewage by sorption
    • C02F1/283Treatment of water, waste water, or sewage by sorption using coal, charred products, or inorganic mixtures containing them
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/28Treatment of water, waste water, or sewage by sorption
    • C02F1/288Treatment of water, waste water, or sewage by sorption using composite sorbents, e.g. coated, impregnated, multi-layered
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F2101/00Nature of the contaminant
    • C02F2101/10Inorganic compounds
    • C02F2101/20Heavy metals or heavy metal compounds
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F2209/00Controlling or monitoring parameters in water treatment
    • C02F2209/08Chemical Oxygen Demand [COD]; Biological Oxygen Demand [BOD]
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F2209/00Controlling or monitoring parameters in water treatment
    • C02F2209/10Solids, e.g. total solids [TS], total suspended solids [TSS] or volatile solids [VS]

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  • Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Hydrology & Water Resources (AREA)
  • Engineering & Computer Science (AREA)
  • Environmental & Geological Engineering (AREA)
  • Water Supply & Treatment (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Solid-Sorbent Or Filter-Aiding Compositions (AREA)
  • Water Treatment By Sorption (AREA)

Abstract

The invention provides an efficient compound desulfurization wastewater treatment agent and a preparation method thereof, wherein the desulfurization wastewater treatment agent comprises the following components: diatomite: 20-30 parts by mass of cement: 5-10 parts by mass of calcium sulfate: 30-50 parts by mass of activated carbon: 5-10 parts by mass of modified zeolite, 10-20 parts by mass of modified bentonite: 10-20 parts by mass. The efficient compound desulfurization wastewater treatment agent and the preparation method thereof have the advantages of good treatment effect, low treatment cost, low operation cost and simplicity in operation.

Description

Efficient composite desulfurization wastewater treatment agent and preparation method thereof
[ technical field ] A method for producing a semiconductor device
The invention relates to the technical field of preparation of medicaments in thermal power plants, in particular to a high-efficiency compound type desulfurization wastewater treatment medicament and a preparation method thereof.
[ background of the invention ]
The traditional three-header chemical precipitation process of the power plant has various chemical agents, complex process flow and unqualified effluent quality under most conditions.
After the release of the standard DL/T997-2006 in the power industry, a plurality of power plants adopt a 'triple box' dosing process, but few projects which can successfully and stably operate exist, and a plurality of devices are in a resting state. The reason is mainly as follows:
1, for polymeric flocculant, aluminum salt or ferric salt, the pH value of the wastewater has a large influence on the treatment effect, and the fluctuation of the pH value can seriously influence the reaction effect of the flocculant.
2, most of the medicaments added into the triple box are required to be diluted and dissolved, and are added by a metering pump. A plurality of premixing devices and dosing devices are needed to be added. And further greatly improves the operation cost, the equipment maintenance cost and the equipment energy consumption.
3, in the traditional treatment process, the reagent needs longer reaction time, but most of the three headers in the power plant are not designed to achieve the reaction time required by the traditional reagent. Resulting in effluent that fails to achieve the desired results.
4, the bed mud after traditional medicament is handled has very big viscidity, can influence the production operation of follow-up desliming equipment to sheet frame desliming equipment is taken as the example, and the mud cake of pressing futilely can't drop to the mud storehouse naturally, needs artifical assistance. And the dehydrated bottom mud contains a large amount of chemical agents and cannot be reused.
Therefore, there is a need for a compound desulfurization wastewater treatment agent and a preparation method thereof for thermal power plants to overcome the deficiencies of the prior art, so as to solve or alleviate one or more of the above problems.
[ summary of the invention ]
In view of the above, the invention provides an efficient compound desulfurization wastewater treatment agent and a preparation method thereof, and the efficient compound desulfurization wastewater treatment agent has the advantages of good treatment effect, low treatment cost, low operation cost and simplicity in operation.
In one aspect, the invention provides an efficient compound desulfurization wastewater treatment agent, which comprises:
diatomite: 20-30 parts by mass of a water-soluble polymer,
cement: 5-10 parts by mass of a stabilizer,
calcium sulfate: 30-50 parts by mass of a water-soluble polymer,
activated carbon: 5-10 parts by mass of a stabilizer,
10-20 parts by mass of modified zeolite,
modified bentonite: 10-20 parts by mass.
The above aspect and any possible implementation manner further provide an implementation manner, wherein the diatomite is seawater diatomite and is used for removing heavy metals from the desulfurization wastewater through adsorption.
The above aspects and any possible implementations further provide an implementation where the cement is a mixture of any one or two of portland cement and high alumina cement mixed in any proportion.
The above aspect and any possible implementation manner further provide an implementation manner, wherein the calcium sulfate is anhydrous calcium sulfate of 100 mesh to 200 mesh.
The above aspect and any possible implementation further provides an implementation, wherein the modified zeolite is formed from 1: soaking zeolite in NaCl in the solid-liquid ratio of 1mol/L for over 12 hr, washing the salt solution on the surface of zeolite, and stoving.
The above aspects and any possible implementations further provide an implementation in which the modified bentonite is an acid-modified bentonite.
The above aspects and any possible implementation manners further provide an implementation manner, wherein the activated carbon is coconut shell activated carbon with a particle size of more than 100 meshes and a water content of less than or equal to 10%.
The above aspects and any possible implementation manners further provide a preparation method of the efficient compound desulfurization wastewater treatment agent, and the preparation method comprises the following steps:
s1: carrying out powder modification on zeolite in medicament raw materials to obtain modified zeolite;
s2: performing powder modification on bentonite in a medicament raw material to obtain modified bentonite;
s3: sequentially adding cement and calcium sulfate into the modified zeolite according to respective proportions, and uniformly mixing to obtain a mixture A;
s4: sequentially adding diatomite and active carbon into the modified bentonite according to respective proportions, and uniformly mixing to obtain a mixture B;
s5: and uniformly mixing the mixture A and the mixture B to finally obtain the desulfurization wastewater treatment agent.
As for the above-mentioned aspect and any possible implementation manner, there is further provided an implementation manner, where the S3 specifically is: and sequentially adding the modified zeolite, the cement and the calcium sulfate into a powder stirrer, uniformly mixing and stirring for 1-2 hours.
As for the above-mentioned aspect and any possible implementation manner, there is further provided an implementation manner, where the S4 specifically is: sequentially adding the modified bentonite, the diatomite and the active carbon into a powder stirrer, uniformly mixing and stirring for 1-2 hours.
Compared with the prior art, the invention can obtain the following technical effects:
1: the invention uses a novel medicament to replace 4-5 medicaments in the original process, and has the advantages of high reaction speed, good treatment effect and greatly reduced medicament cost;
2: the novel medicament adopts a dry powder dosing device, and premixing equipment is not required, so that the cost of dosing equipment, the equipment maintenance cost and the operation cost are greatly reduced;
3: the reaction speed of the novel medicament and the waste water is far faster than that of the traditional medicament, so that the volume of reaction equipment can be greatly reduced, and the manufacturing cost and the occupied area of the equipment are reduced.
4: the novel medicament is composed of natural non-metallic substances, is non-toxic and harmless, so that the settled sludge can enter a gypsum storehouse after being dehydrated for resource utilization, and no heavy metal or other harmful substances overflow through detecting the leachate after the sludge acid leaching experiment, so that the sludge has no secondary pollution to the environment.
5: the inorganic material modification technology mainly takes acid solution and salt solution as modifiers, and the specific surface area and the adsorption capacity of the modified inorganic material are greatly enhanced.
Of course, it is not necessary for any one product in which the invention is practiced to achieve all of the above-described technical effects simultaneously.
[ description of the drawings ]
In order to more clearly illustrate the technical solutions of the embodiments of the present invention, the drawings needed to be used in the embodiments will be briefly described below, and it is obvious that the drawings in the following description are only some embodiments of the present invention, and it is obvious for those skilled in the art to obtain other drawings based on these drawings without creative efforts.
FIG. 1 is a flow chart of a method for preparing a reagent for treating desulfurization waste water according to an embodiment of the present invention.
[ detailed description ] embodiments
For better understanding of the technical solutions of the present invention, the following detailed descriptions of the embodiments of the present invention are provided with reference to the accompanying drawings.
It should be understood that the described embodiments are only some embodiments of the invention, and not all embodiments. All other embodiments, which can be derived by a person skilled in the art from the embodiments given herein without making any creative effort, shall fall within the protection scope of the present invention.
The terminology used in the embodiments of the invention is for the purpose of describing particular embodiments only and is not intended to be limiting of the invention. As used in the examples of the present invention and the appended claims, the singular forms "a," "an," and "the" are intended to include the plural forms as well, unless the context clearly indicates otherwise.
The invention provides a high-efficiency compound desulfurization wastewater treatment agent, which comprises the following components:
diatomite: 20-30 parts by mass of a water-soluble polymer,
cement: 5-10 parts by mass of a stabilizer,
calcium sulfate: 30-50 parts by mass of a water-soluble polymer,
activated carbon: 5-10 parts by mass of a stabilizer,
10-20 parts by mass of modified zeolite,
modified bentonite: 10-20 parts by mass.
The kieselguhr is seawater kieselguhr and is used for removing heavy metals in the desulfurization wastewater through adsorption, the cement is any one of Portland cement and high-alumina cement or a mixture mixed in any proportion, the calcium sulfate is anhydrous calcium sulfate of 100 meshes, and the modified zeolite is prepared from the following components in percentage by weight: fully soaking zeolite for more than 12 hours by using 1mol/L NaCl with the solid-liquid ratio of 20, cleaning a salt solution on the surface of the zeolite, and drying to obtain the modified bentonite, wherein the modified bentonite is acid modified bentonite, and the activated carbon is coconut shell activated carbon with the particle size of more than 100 meshes and the water content of less than or equal to 10%.
The invention also provides a preparation method of the efficient compound desulfurization wastewater treatment agent, a basic process flow diagram of the preparation method is shown in figure 1, and the preparation method comprises the following steps:
s1: carrying out powder modification on zeolite in medicament raw materials to obtain modified zeolite;
s2: performing powder modification on bentonite in a medicament raw material to obtain modified bentonite;
s3: sequentially adding cement and calcium sulfate into the modified zeolite according to respective proportions, and uniformly mixing to obtain a mixture A;
s4: sequentially adding diatomite and active carbon into the modified bentonite according to respective proportions, and uniformly mixing to obtain a mixture B;
s5: and uniformly mixing the mixture A and the mixture B to finally obtain the desulfurization wastewater treatment agent.
The S3 specifically includes: and sequentially adding the modified zeolite, the cement and the calcium sulfate into a powder stirrer, uniformly mixing and stirring for 1-2 hours.
The S4 specifically includes: sequentially adding the modified bentonite, the diatomite and the active carbon into a powder stirrer, uniformly mixing and stirring for 1-2 hours
The technical principle of powder modification in S3 and S4 in the invention is as follows:
the zeolite in the raw material of the medicament is subjected to powder modification, the zeolite is a general name of a porous water-containing aluminosilicate mineral with a frame structure, in the framework of the material, negative points on anion lattices and positive charge centers of balancing cations are not overlapped in space, so that large electrostatic attraction force is generated among molecules, a plurality of holes and channels with uniform sizes are formed in the material, and the holes are connected with each other through the channels, so that the material has a large specific surface area (400-800 square meters per gram) and good adsorption performance. The ion exchange capacity of the zeolite can be greatly improved by modifying the zeolite by a physical and chemical method, and the adsorption performance of the raw material modified by salt is improved by more than 15-20%.
The bentonite in the raw materials of the medicament is subjected to powder modification, the bentonite is hydrous clay mineral mainly containing montmorillonite, and has a layered crystal structure, cations among layers of the hydrous clay mineral are easy to exchange, and the bentonite has a large ion exchange capacity. After the bentonite is modified by acidification, the specific surface area of the material is increased, and impurities such as soluble substances, mixed organic matters and the like distributed in the pore canal of the material can be removed by adding acid, so that the pore canal of the material is dredged, and the diffusion of adsorbate molecules is facilitated, and meanwhile, because the radius of hydrogen atoms is smaller than the radius of atoms such as sodium ions, potassium ions, magnesium ions, calcium ions and the like, the hydrogen atoms with smaller volume ionized by the modified acid can replace various cations between bentonite layers, so that the pore volume is increased, the original interlayer bonding force is weakened, the layered crystal lattice is cracked, the pore canal is dredged, and the adsorption performance is improved by more than 40-50%.
After the desulfurization wastewater treatment agent prepared by the invention is put into use, the results are as follows:
1. after the novel medicament is used, the removal rate of suspended matters in the wastewater reaches over 99 percent, the removal rate of heavy metals reaches over 98 percent, and the removal rate of COD is over 40 percent;
2. the added medicaments of the system are changed from the original 5 medicaments to only one medicament;
3. the reaction speed of the medicament is improved by more than one time compared with the traditional 'triple-box' medicament.
4. The water quality of the desulfurization wastewater treated by the medicament completely reaches the DL/T997-2006 standard
Figure BDA0002813926100000071
Figure BDA0002813926100000081
The efficient compound desulfurization wastewater treatment agent and the preparation method thereof provided by the embodiment of the application are introduced in detail. The above description of the embodiments is only for the purpose of helping to understand the method of the present application and its core ideas; meanwhile, for a person skilled in the art, according to the idea of the present application, there may be variations in the specific embodiments and the application scope, and in summary, the content of the present specification should not be construed as a limitation to the present application.
As used in the specification and claims, certain terms are used to refer to particular components. As one skilled in the art will appreciate, manufacturers may refer to a component by different names. This specification and claims do not intend to distinguish between components that differ in name but not function. In the following description and in the claims, the terms "include" and "comprise" are used in an open-ended fashion, and thus should be interpreted to mean "include, but not limited to. "substantially" means within an acceptable error range, and a person skilled in the art can solve the technical problem within a certain error range to substantially achieve the technical effect. The description which follows is a preferred embodiment of the present application, but is made for the purpose of illustrating the general principles of the application and not for the purpose of limiting the scope of the application. The protection scope of the present application shall be subject to the definitions of the appended claims.
It is also noted that the terms "comprises," "comprising," or any other variation thereof, are intended to cover a non-exclusive inclusion, such that a good or system that comprises a list of elements does not include only those elements but may include other elements not expressly listed or inherent to such good or system. Without further limitation, an element defined by the phrase "comprising an … …" does not exclude the presence of other like elements in a commodity or system that includes the element.
It should be understood that the term "and/or" as used herein is merely one type of association that describes an associated object, meaning that three relationships may exist, e.g., a and/or B may mean: a exists alone, A and B exist simultaneously, and B exists alone. In addition, the character "/" herein generally indicates that the former and latter related objects are in an "or" relationship.
The foregoing description shows and describes several preferred embodiments of the present application, but as aforementioned, it is to be understood that the application is not limited to the forms disclosed herein, but is not to be construed as excluding other embodiments and is capable of use in various other combinations, modifications, and environments and is capable of changes within the scope of the application as described herein, commensurate with the above teachings, or the skill or knowledge of the relevant art. And that modifications and variations may be effected by those skilled in the art without departing from the spirit and scope of the application, which is to be protected by the claims appended hereto.

Claims (10)

1. The high-efficiency compound desulfurization wastewater treatment agent is characterized by comprising the following components in parts by weight:
diatomite: 20-30 parts by mass of a water-soluble polymer,
cement: 5-10 parts by mass of a stabilizer,
calcium sulfate: 30-50 parts by mass of a water-soluble polymer,
activated carbon: 5-10 parts by mass of a stabilizer,
10-20 parts by mass of modified zeolite,
modified bentonite: 10-20 parts by mass.
2. The desulfurization wastewater treatment chemical according to claim 1, wherein the diatomaceous earth is seawater diatomaceous earth, and is used for removing heavy metals from desulfurization wastewater by adsorption.
3. The desulfurization wastewater treatment agent according to claim 1, wherein the cement is a mixture of any one or two of portland cement and high-alumina cement mixed in any ratio.
4. The desulfurization wastewater treatment agent according to claim 1, wherein the calcium sulfate is anhydrous calcium sulfate of between 100 mesh and 200 mesh.
5. The desulfurization wastewater treatment agent according to claim 1, wherein the modified zeolite is composed of 1: soaking zeolite in NaCl in the solid-liquid ratio of 1mol/L for over 12 hr, washing the salt solution on the surface of zeolite, and stoving.
6. The desulfurization wastewater treatment chemical according to claim 1, wherein the modified bentonite is acid-modified bentonite.
7. The desulfurization wastewater treatment agent according to claim 1, wherein the activated carbon is coconut shell activated carbon with a particle size of 100 meshes or more and a water content of 10% or less.
8. A method for preparing a high-efficiency compound desulfurization wastewater treatment agent, which comprises the desulfurization wastewater treatment agent of any one of claims 1 to 7, and is characterized by comprising the following steps:
s1: carrying out powder modification on zeolite in medicament raw materials to obtain modified zeolite;
s2: performing powder modification on bentonite in a medicament raw material to obtain modified bentonite;
s3: sequentially adding cement and calcium sulfate into the modified zeolite, and uniformly mixing to obtain a mixture A;
s4: sequentially adding diatomite and active carbon into the modified bentonite, and uniformly mixing to obtain a mixture B;
s5: and uniformly mixing the mixture A and the mixture B to finally obtain the desulfurization wastewater treatment agent.
9. The preparation method according to claim 8, wherein the S3 is specifically: and sequentially adding the modified zeolite, the cement and the calcium sulfate into a powder stirrer, uniformly mixing and stirring for 1-2 hours.
10. The desulfurization wastewater treatment agent according to claim 1, wherein the S4 is specifically: sequentially adding the modified bentonite, the diatomite and the active carbon into a powder stirrer, uniformly mixing and stirring for 1-2 hours.
CN202011393993.5A 2020-12-02 2020-12-02 Efficient composite desulfurization wastewater treatment agent and preparation method thereof Pending CN112479282A (en)

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN116081771A (en) * 2022-12-09 2023-05-09 大唐东北电力试验研究院有限公司 An integrated desulfurization wastewater treatment agent and its preparation method

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CN108557976A (en) * 2018-04-20 2018-09-21 东莞市顶盛环保科技有限公司 A kind of high-efficiency sewage ammonia nitrogen removal agent
CN109231334A (en) * 2018-08-28 2019-01-18 浙江正洁环境科技有限公司 A kind of waste water integrated treatment medicament and its application
CN109704446A (en) * 2019-01-10 2019-05-03 四川大学 A method for efficiently removing phosphorus in eutrophic water
CN110228831A (en) * 2019-06-18 2019-09-13 天津伟创园林绿化有限公司 A kind of water remediation agent administered for black and odorous water containing natural mineral matter

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20170101332A1 (en) * 2008-02-14 2017-04-13 Soane Mining, Llc Systems and methods for removing finely dispersed particulate matter from a fluid stream
CN105883995A (en) * 2016-06-08 2016-08-24 山东巴博尔环保科技有限公司 Novel magnesium-based quick-setting material and preparation method and application thereof
CN108557976A (en) * 2018-04-20 2018-09-21 东莞市顶盛环保科技有限公司 A kind of high-efficiency sewage ammonia nitrogen removal agent
CN109231334A (en) * 2018-08-28 2019-01-18 浙江正洁环境科技有限公司 A kind of waste water integrated treatment medicament and its application
CN109704446A (en) * 2019-01-10 2019-05-03 四川大学 A method for efficiently removing phosphorus in eutrophic water
CN110228831A (en) * 2019-06-18 2019-09-13 天津伟创园林绿化有限公司 A kind of water remediation agent administered for black and odorous water containing natural mineral matter

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN116081771A (en) * 2022-12-09 2023-05-09 大唐东北电力试验研究院有限公司 An integrated desulfurization wastewater treatment agent and its preparation method

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Application publication date: 20210312