[go: up one dir, main page]

CN113621341A - Special high-temperature repairing agent for leaking stoppage of drying cylinder - Google Patents

Special high-temperature repairing agent for leaking stoppage of drying cylinder Download PDF

Info

Publication number
CN113621341A
CN113621341A CN202111061368.5A CN202111061368A CN113621341A CN 113621341 A CN113621341 A CN 113621341A CN 202111061368 A CN202111061368 A CN 202111061368A CN 113621341 A CN113621341 A CN 113621341A
Authority
CN
China
Prior art keywords
temperature
epoxy resin
repairing agent
filler
carbon black
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
CN202111061368.5A
Other languages
Chinese (zh)
Inventor
张春祥
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Zhenjiang Xingxing Technology Co ltd
Original Assignee
Zhenjiang Xingxing Technology Co ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Zhenjiang Xingxing Technology Co ltd filed Critical Zhenjiang Xingxing Technology Co ltd
Priority to CN202111061368.5A priority Critical patent/CN113621341A/en
Publication of CN113621341A publication Critical patent/CN113621341A/en
Pending legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J183/00Adhesives based on macromolecular compounds obtained by reactions forming in the main chain of the macromolecule a linkage containing silicon, with or without sulfur, nitrogen, oxygen, or carbon only; Adhesives based on derivatives of such polymers
    • C09J183/04Polysiloxanes
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J11/00Features of adhesives not provided for in group C09J9/00, e.g. additives
    • C09J11/02Non-macromolecular additives
    • C09J11/04Non-macromolecular additives inorganic
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J11/00Features of adhesives not provided for in group C09J9/00, e.g. additives
    • C09J11/08Macromolecular additives
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/18Oxygen-containing compounds, e.g. metal carbonyls
    • C08K3/20Oxides; Hydroxides
    • C08K3/22Oxides; Hydroxides of metals
    • C08K2003/2227Oxides; Hydroxides of metals of aluminium
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L2201/00Properties
    • C08L2201/08Stabilised against heat, light or radiation or oxydation
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L2205/00Polymer mixtures characterised by other features
    • C08L2205/02Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group
    • C08L2205/025Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group containing two or more polymers of the same hierarchy C08L, and differing only in parameters such as density, comonomer content, molecular weight, structure

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Compositions Of Macromolecular Compounds (AREA)

Abstract

The invention relates to a special high-temperature repairing agent for leaking stoppage of a drying cylinder, which consists of polysiloxane, white carbon black, a filler and high-temperature epoxy resin; the filler is inorganic nonmetallic particles and/or organic filler, the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and solvent, polysiloxane is taken into white carbon black and the filler is sheared, the high-temperature epoxy resin is added according to the following formulation principle and is uniformly stirred, then the rust remover can be adopted to treat and cool the oxide layer of the cylinder body and the cylinder cover and polish the combination part of the cylinder body and the cylinder cover, the high-temperature repairing agent is uniformly coated at the defect part, the high-temperature repairing agent is pressurized and compact after being solidified, and the high-temperature repairing agent is coated for the second time and solidified, so that the heat resistance is obviously improved, the high-adhesion property and the solidification toughness which can resist the temperature higher than 280 ℃ are achieved, the elasticity and the high-temperature sealing property are good, the electric insulation property is high, the fatigue strength is good, the high-temperature-resistant sealing and caulking can be used for plane sealing and repairing in a drying cylinder, especially for repairing in the drying cylinder, and the drying cylinder can adapt to the thermal expansion and cold contraction under different temperatures.

Description

Special high-temperature repairing agent for leaking stoppage of drying cylinder
Technical Field
The invention relates to a special high-temperature repairing agent for leakage stoppage of a drying cylinder, belonging to the technical field of high-temperature compact repairing materials of drying cylinders.
Background
The drying cylinder is made of cast iron and the two ends of the cylindrical cylinder body are provided with the drying structures of the cylinder covers, steam is introduced in the operation process, saturated steam introduced from the steam joint is condensed in the drying cylinder, condensed water is attached to the inner surface of the drying cylinder due to the centrifugal force generated by the rotation of the drying cylinder, the accumulation of water rings is avoided through siphon drainage, and the temperature of the drying cylinder is raised due to the heat released by the steam, so that a product which runs on the surface of the roller shell is dried and ironed, the finishing effect is achieved, and the drying cylinder is widely applied to the papermaking industry. The plasticity, strength limit and corrosion resistance of the cast iron material of the drying cylinder are poor and are influenced by cold and hot temperature, local uneven heating, rotating operation tensile stress and other factors, the cylinder body is easy to generate cracks, abrasion, corrosion, ablation and the like, and if the cylinder body is not repaired in time, the structural damage is aggravated, and even steam and water leakage are generated to influence production. The repair welding method has high professional requirements on operators and tools, high-temperature operation environment and welding flux in a cylinder are not beneficial to leakage repair of a drying cylinder, and the problems of leaving welding seams, holes, solid impurities and the like exist.
Disclosure of Invention
The invention aims to provide the special high-temperature repairing agent for the leakage stoppage of the drying cylinder, which obviously improves the temperature resistance, the metal adhesion and the curing toughness, has good elasticity and high-temperature sealing performance, high electrical insulation performance and good fatigue resistance, can be used for plane sealing and caulking under high-temperature working conditions, particularly repairing in the drying cylinder, and can adapt to the thermal expansion and cold contraction of the drying cylinder at different temperatures.
The invention is realized by the following technical scheme:
the special high-temperature repairing agent for dryer leakage stoppage is prepared from polysiloxane, white carbon black, filler and high-temperature epoxy resin according to the mass ratio of 35-70:5-10: 1-20: 2-25;
the special high-temperature repairing agent for the dryer leakage stoppage is characterized in that the polysiloxane is one or more of polydimethylsiloxane, hydroxyl-terminated linear polydimethylsiloxane, cyclic polydimethylsiloxane and divinyl polydimethylsiloxane; the white carbon black is hydrophobic white carbon black; the filler is inorganic non-metal particles and/or organic filler, the inorganic non-metal particles are one or more of nano silicon carbide, nano calcium carbonate, talcum powder, nano alumina, nano titanium oxide, kaolin and mica powder, the inorganic non-metal particles further comprise hydrophobic surface treatment particles, and the organic filler is one or more of styrene acrylonitrile copolymer particles, acrylonitrile-butadiene-styrene copolymer particles and polyvinyl butyral powder.
The special high-temperature repairing agent for leaking stoppage of the drying cylinder is characterized in that the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and a solvent in a mass ratio of 50-65: 5-15: 4-8: 10-20; the glycidyl ether type epoxy resin is one or more of bisphenol A type epoxy resin, phenol formaldehyde type epoxy resin, o-benzaldehyde type epoxy resin, resorcinol formaldehyde type epoxy resin, trihydroxyphenyl methane type epoxy resin and polyalcohol glycidyl ether type epoxy resin, the thermoplastic resin is one or more of bismaleimide resin BMI, polyimide resin PI and polyetherimide PEI, the diamine is one or more of diaminodiphenylmethane DDM, diaminodiphenyl ether DDE and diaminodiphenyl sulfone DDS, and the solvent is acetone, methanol or xylene.
The special high-temperature repairing agent for leaking stoppage of the drying cylinder is constructed at the temperature of more than or equal to 15 ℃ and the humidity of less than or equal to 90% when the high-temperature repairing agent is used for repairing defects in the drying cylinder, and is prepared by treating and cooling an oxide layer of the cylinder body and the cylinder cover by using a rust remover, polishing a joint part of the cylinder body and the cylinder cover, uniformly coating the high-temperature repairing agent on the defect, pressurizing and compacting after curing, coating the high-temperature repairing agent for the second time and curing for 8-12 hours.
The preparation method of the special high-temperature repairing agent for dryer leaking stoppage comprises the following steps: taking polyorganosiloxane into white carbon black and filler, shearing at the speed of 600 plus 1000rpm for 20-40min, adding high-temperature epoxy resin according to the random mixing principle, and uniformly stirring to prepare the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 35-70:5-10: 1-20: 2 to 25;
the white carbon black/filler is subjected to hydrophobic surface treatment, and the treatment steps are as follows: taking precipitated silica/filler and water, stirring for 5-10min, adding a silane coupling agent, dissolving in a solvent, stirring for 10-30min, aging for 1-2h, filtering, taking a filter cake, washing and drying with ethanol to obtain hydrophobic silica/hydrophobic surface filler, wherein the mass ratio of the precipitated silica/filler, water, the silane coupling agent and the solvent is 80-90: 100-150:2-4:12-30, wherein the silane coupling agent is one or more of KH560, KH792 and DL602, and the solvent is acetone, methanol or benzene;
the high-temperature epoxy resin is prepared by stirring and preheating glycidyl ether epoxy resin and a solvent, then sequentially adding thermoplastic resin and diamine, and stirring at 60-75 ℃ and 200-400rpm for 20-30 min.
The invention has the beneficial effects that:
the polyorganosiloxane has smaller surface tension, higher surface activity, no corrosion to metal, low viscosity-temperature coefficient, water permeability and water absorption limiting and reducing capability after the solid surface is treated, and higher compression resistance; white carbon black is adopted for reinforcing and filling, so that a large number of chemical interfaces can be generated with polysiloxane and epoxy resin, a viscous rheological effect is endowed, crack propagation is prevented, and the stress at definite elongation, the tear strength, the tensile strength and the wear resistance are improved; through filling modification of filler particles, the sliding deformation tension is increased, uniform stress is buffered, overall cracking of the material is reduced, the strength is improved, and the softening starting temperature and the chemical corrosion resistance of the repairing agent are improved;
the epoxy resin system has high adhesive force of large active epoxy groups and polar groups to cast iron metal polar materials, epoxy condensate has good cohesive strength and adhesive strength, the reduction of curing shrinkage is favorable for improving the adhesive strength, the molecular flexibility is improved through modification, the high-temperature resistance is better, the epoxy resin system and polyorganosiloxane form two-component curing, high-performance reaction curing room temperature vulcanized rubber RTV, the long-term temperature resistance is 350 ℃, the instant temperature resistance is 450 ℃, the elasticity and the high-temperature sealing performance are good, the electrical insulation performance is high, the fatigue strength is good, the epoxy resin system can be used for plane sealing and caulking under high-temperature working conditions, particularly in-cylinder repairing of drying cylinders, the epoxy resin system has strong adhesion with the temperature resistance of more than 280 ℃, and the epoxy resin system has certain toughness after curing, and can be suitable for drying cylinders with cold and heat shrinkage under different temperatures.
Detailed Description
The following examples further illustrate embodiments of the present invention.
Example 1
The preparation method of the special high-temperature repairing agent for dryer leak stoppage comprises the following steps:
adding white carbon black and a filler into polyorganosiloxane, shearing at 700rpm for 30min, adding high-temperature epoxy resin according to a random mixing principle, and uniformly stirring to obtain the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 68:6: 15: 15;
the polyorganosiloxane is polydimethylsiloxane;
the white carbon black is hydrophobic white carbon black;
the filler is inorganic non-metal particles, and the inorganic non-metal particles are composed of nano silicon carbide, talcum powder, nano aluminum oxide and mica powder according to the mass ratio of 1:1:1: 2;
taking precipitated silica/filler and water, stirring for 8min, adding a silane coupling agent, dissolving in a solvent, stirring for 20min, aging for 2h, filtering, taking a filter cake, washing and drying by using ethanol to obtain hydrophobic silica/hydrophobic surface filler, wherein the mass ratio of the precipitated silica/filler, the water, the silane coupling agent and the solvent is 85: 120:3:16, wherein the silane coupling agent is KH560, and the solvent is acetone;
the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and a solvent in a mass ratio of 58: 20: 6: 13;
the glycidyl ether epoxy resin is bisphenol A epoxy resin and phenol formaldehyde epoxy resin in a mass ratio of 2:1, the thermoplastic resin is bismaleimide resin BMI, the diamine is diaminodiphenylmethane DDM, and diaminodiphenyl ether DDE in a mass ratio of 2:1, wherein the solvent is acetone;
the high-temperature epoxy resin is prepared by stirring glycidyl ether epoxy resin and a solvent, preheating, sequentially adding thermoplastic resin and diamine, and stirring at 72 ℃ and 350rpm for 25 min.
Example 2
The preparation method of the special high-temperature repairing agent for dryer leak stoppage comprises the following steps:
adding white carbon black and a filler into polyorganosiloxane, shearing at 700rpm for 30min, adding high-temperature epoxy resin according to a random mixing principle, and uniformly stirring to obtain the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 45:7: 15: 8;
the polyorganosiloxane consists of hydroxyl-terminated linear polydimethylsiloxane and cyclic polydimethylsiloxane in a mass ratio of 2: 1;
the white carbon black is hydrophobic white carbon black;
the filler is composed of inorganic non-metal particles and an organic filler according to the mass ratio of 2:1, the inorganic non-metal particles are composed of nano calcium carbonate, nano alumina and kaolin according to the mass ratio of 1:1:2, and the organic filler is hot-melt styrene acrylonitrile copolymer particles;
taking precipitated silica/inorganic non-metallic filler and water, stirring for 8min, adding a silane coupling agent, dissolving in a solvent, stirring for 22min, aging for 1.5h, filtering, taking a filter cake, washing and drying with ethanol to obtain hydrophobic silica/hydrophobic surface inorganic non-metallic filler, wherein the mass ratio of the precipitated silica/inorganic non-metallic filler, the water, the silane coupling agent and the solvent is 83: 110:3:18, wherein the silane coupling agent is KH792, and the solvent is acetone;
the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and a solvent in a mass ratio of 58: 9: 6: 13;
the glycidyl ether type epoxy resin is composed of phenol formaldehyde type epoxy resin, o-benzaldehyde type epoxy resin and polyhydric alcohol glycidyl ether type epoxy resin according to the mass ratio of 1:1:2, the thermoplastic resin is polyimide resin PI, the diamine is diaminodiphenyl ether DDE and diaminodiphenyl sulfone DDS according to the mass ratio of 2:1, and the solvent is composed of acetone and methanol according to the mass ratio of 2: 1;
the high-temperature epoxy resin is prepared by stirring glycidyl ether epoxy resin and a solvent, preheating, sequentially adding thermoplastic resin and diamine, and stirring at 68 ℃ and 350rpm for 25 min.
Example 3
The preparation method of the special high-temperature repairing agent for dryer leak stoppage comprises the following steps:
adding the polyorganosiloxane into the white carbon black and the filler, shearing for 35min at the speed of 600-1000rpm, adding the high-temperature epoxy resin according to the random mixing principle, and uniformly stirring to prepare the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 65:8: 15: 17;
the polyorganosiloxane is composed of hydroxyl-terminated linear polydimethylsiloxane and divinyl polydimethylsiloxane in a mass ratio of 1: 2;
the white carbon black is hydrophobic white carbon black;
the filler is inorganic non-metal particles and an organic filler, the inorganic non-metal particles are composed of nano silicon carbide, nano calcium carbonate, nano aluminum oxide and nano titanium oxide according to the mass ratio of 2:1:1:1, and the organic filler is composed of hot-melt acrylonitrile-butadiene-styrene copolymer particles and polyvinyl butyral powder according to the mass ratio of 1: 1;
taking precipitated white carbon black/inorganic non-metallic particle filler and water, stirring for 8min, adding a silane coupling agent, dissolving in a solvent, stirring for 18min, aging for 2h, filtering, taking a filter cake, washing and drying with ethanol to obtain hydrophobic white carbon black/hydrophobic surface filler, wherein the mass ratio of the precipitated white carbon black/inorganic non-metallic particle filler, the water, the silane coupling agent and the solvent is 83: 146:3:21, wherein the silane coupling agent is KH792, and the solvent is methanol;
the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and a solvent in a mass ratio of 57: 11: 6: 16;
the glycidyl ether epoxy resin is composed of resorcinol formaldehyde epoxy resin and trihydroxyphenyl methane epoxy resin according to the mass ratio of 2:1, the thermoplastic resin is composed of polyimide resin PI and polyetherimide PEI according to the mass ratio of 2:1, the diamine is diaminodiphenylmethane DDM, and the solvent is xylene;
the high-temperature epoxy resin is prepared by stirring glycidyl ether epoxy resin and a solvent, preheating, sequentially adding thermoplastic resin and diamine, and stirring at 72 ℃ and 350rpm for 25 min.
Example 4
The preparation method of the special high-temperature repairing agent for dryer leak stoppage comprises the following steps:
adding white carbon black and a filler into polyorganosiloxane, shearing at 650rpm for 30min, adding high-temperature epoxy resin according to a random mixing principle, and uniformly stirring to obtain the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 38:11: 13: 17;
the polysiloxane is composed of polydimethylsiloxane and divinyl polydimethylsiloxane in a mass ratio of 1: 1;
the filler is inorganic non-metal particles, and the inorganic non-metal particles are composed of nano calcium carbonate, talcum powder, nano alumina, kaolin and mica powder according to a mass ratio of 2:1:1: 2;
stirring filler and water for 6min, adding a silane coupling agent, dissolving in a solvent, stirring for 20min, aging for 1.5h, filtering, washing a filter cake with ethanol, and drying to obtain the hydrophobic surface filler, wherein the mass ratio of the filler to the water to the silane coupling agent to the solvent is 82: 118:3:17, wherein the silane coupling agent is DL602, and the solvent is acetone;
the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and a solvent in a mass ratio of 53: 11: 6: 16;
the glycidyl ether type epoxy resin is bisphenol A type epoxy resin, trihydroxyphenyl methane type epoxy resin and polyhydric alcohol glycidyl ether type epoxy resin according to the mass ratio of 2:1:1, the thermoplastic resin is bismaleimide resin BMI and polyimide resin PI according to the mass ratio of 2:1, the diamine is diaminodiphenyl methane DDM and diaminodiphenyl sulfone DDS according to the mass ratio of 2:1, and the solvent is acetone and xylene according to the mass ratio of 2: 1;
the high-temperature epoxy resin is prepared by stirring glycidyl ether epoxy resin and a solvent, preheating, sequentially adding thermoplastic resin and diamine, and stirring at 65 ℃ and 320rpm for 25 min.
The high-temperature repairing agent prepared in the embodiments 1-4 and a commercially available metal repairing agent (poly force JL-101) are used as a comparative example for repairing defects in a drying cylinder, when the defects in the drying cylinder are repaired, construction is carried out at a temperature of more than or equal to 15 ℃ and a humidity of less than or equal to 90%, a rust remover is used for treating a cooling cylinder body and a cylinder cover oxide layer, grinding a combination part of a cylinder body and a cylinder cover, uniformly coating the high-temperature repairing agent on the defect, pressurizing and compacting after curing, and coating the high-temperature repairing agent for the second time, and the detection results of the mechanical property and the curing property (a shearing sample is cured at 23 +/-2 ℃ for 21 days, and the side view temperature is 23 +/-2 ℃) are as follows:
Figure BDA0003256520700000081
the polyorganosiloxane can be used as an adhesive component for bonding metal, has smaller surface tension and higher surface activity, is non-corrosive and nontoxic to metal, has higher Si-O bond energy, excellent heat resistance and oxidation resistance, has low viscosity-temperature coefficient of interaction between silicone oil molecules-small change of viscosity with temperature, and Si-H bond crosslinking into a macromolecular hydrophobic structure, so that the water permeability and water absorption can be limited and reduced after the surface of a solid is treated, and the compression resistance is higher;
the polydimethylsiloxane PDMS is a dimethyl polymer organic silicon compound, and has the performances of good high and low temperature resistance, high hydrophobicity, good air permeability, excellent weather resistance, moisture resistance, insulativity, physiological inertia, corrosion resistance, radiation resistance and the like; the hydroxyl-terminated linear polydimethylsiloxane belongs to hydroxyl silicone oil, and has the characteristics of low viscosity, water resistance and methyl silicone oil; the cyclic polydimethylsiloxane belongs to cyclopentasiloxane silicone oil and has high compatibility; the divinyl polydimethylsiloxane is vinyl-terminated silicone oil, has good activity, can be subjected to crosslinking addition reaction with hydrogen-containing silicone oil to obtain a net structure, and improves the high-temperature resistance;
white carbon black is adopted for reinforcing and filling, so that a large number of chemical interfaces can be generated with polysiloxane and epoxy resin, a viscous rheological effect is endowed, crack propagation is prevented, and the stress at definite elongation, the tear strength, the tensile strength and the wear resistance are improved;
the white carbon black prepared by the precipitation method is prepared by the precipitation reaction of sodium silicate and inorganic acid, an acid area exists, the outer surfaces of inner polysiloxane and active silanol groups are hydrophilic, the infiltration and dispersion uniformity in an organic phase are influenced, the surface hydrophobicity of the white carbon black is modified, the silane coupling agent is one or more of KH 560-gamma-glycidoxypropyltrimethoxysilane, KH792-N- (beta-aminoethyl) -gamma-aminopropyl trimethyl (ethyl) oxysilane and DL 602-N-beta- (aminoethyl) -gamma-aminopropyl methyl dimethoxysilane, the hydroxyl on the surface of the white carbon black is hydrolyzed with the silane coupling agent to form hydrogen bonds under the wet modification, and the silane coupling agent is further dehydrated and condensed under the heating and drying conditions to cover the surface of the white carbon black, reduce the hydroxyl content and present the hydrophobic surface characteristic, the dispersibility is improved, and agglomeration is avoided;
the filler particles are filled and modified, the operation is easy, the adhesive process performance and the durability are improved through the filler, the proper viscosity is obtained, the reinforcing repairing agent moves during stretching, the sliding deformation tension is increased, the effect of buffering uniform stress is achieved, the overall breakage of the material is reduced, the strength is improved, the softening starting temperature of the repairing agent is improved, and the chemical corrosion resistance is improved;
the inorganic nonmetal particles in the filler have small size, the surface atomic number accounts for the total specific gravity of the particles, the surface activity is larger due to the unsaturation of the surface atoms, the intermolecular acting force is improved due to the surface effect, the acting force which is larger than the van der Waals force is formed on the interface of the epoxy resin, the polyorganosiloxane and the nano particles, so that the epoxy resin, the polyorganosiloxane and the nano particles have better compatibility, and the repair agent absorbs energy when being stressed to generate cracks, and improves the wear resistance, the tensile strength, the impact strength, the thermal decomposition temperature and the thermal stability;
the addition of nano silicon carbide, nano calcium carbonate, talcum powder and kaolin in the inorganic nonmetal particles can improve the hardness and strength after curing, the addition of nano aluminum oxide can improve the bonding strength and heat resistance, the addition of nano titanium oxide has covering power and can accelerate the curing reaction, and the addition of mica powder can improve the curing water resistance and promote the curing reaction; the inorganic non-metal particles are subjected to hydrophobic surface treatment to improve the dispersibility;
the organic filler can avoid the situation that the inorganic filler is unevenly dispersed and lacks chemical bonding force, so that the tearing strength is reduced when the bearing capacity is improved, the organic filler is used for filling and dispersing, and the strength, the heat resistance, the flexibility and the tearing strength of the repairing agent are improved by chemical acting force, and styrene acrylonitrile copolymer particles SAN in the organic filler have excellent hardness, rigidity, dimensional stability and higher bearing capacity; the acrylonitrile-butadiene-styrene copolymer particles ABS have high strength, good toughness and easy processing and forming; the polyvinyl butyral PVB is combined with thermosetting epoxy resin to improve chemical resistance, elasticity, toughness and coating hardness;
polar groups such as large active epoxy groups, amine bonds, ester bonds, hydroxyl groups and the like in the epoxy resin curing system endow the epoxy cured material with high adhesive force to the cast iron metal polar material, the cohesive strength and the adhesive strength of the epoxy cured material are good, the curing shrinkage is small, the adhesive strength is improved, low-molecular volatile matters are not generated, the process performance is excellent, and the chemical stability is good; the distance between double bonds is increased by the addition reaction of diamine and thermoplastic resin and chain extension, the reaction of active hydrogen and epoxy groups is reduced, the molecular flexibility is improved, the crosslinking density of a cured product is reduced, and the modified epoxy resin has better high-temperature resistance;
glycidyl ether epoxy resin is used as matrix resin, wherein bisphenol A epoxy resin-diphenol propane epoxy resin contains hydroxyl and ether bonds, and has high cohesive force and adhesion; the phenol formaldehyde type epoxy resin, the o-benzaldehyde type epoxy resin-phenolic aldehyde polyfunctional group epoxy resin contains more than two epoxy groups, and the cured product has high crosslinking density and high thermal stability; the cured resorcinol type epoxy resin, resorcinol formaldehyde type epoxy resin-polyhydroxy phenol glycidyl ether type epoxy resin have high heat deformation temperature and rigidity; trihydroxyphenyl methane type epoxy resin and polyhydric alcohol glycidyl ether type epoxy resin contain two or more epoxy groups, have low viscosity and are flexible; the thermoplastic resin is a bismaleimide resin BMI-bifunctional compound with an active end group, has the fluidity similar to that of epoxy resin, and polyimide resin PI-polymer with a main chain containing imide groups and polyetherimide PEI-has excellent thermal stability and high temperature resistance; diaminodiphenylmethane DDM-methylene in diamine has high thermal oxidation stability, diaminodiphenyl ether DDE-is introduced into flexible ether bond, and diaminodiphenyl sulfone DDS-is introduced into rigid sulfone group, so that the heat resistance and the shock resistance of the resin are improved;
the room temperature vulcanized rubber RTV is cured by two components of polyorganosiloxane, has high performance and reaction curing, has simple curing process, can reduce the internal stress of epoxy resin, forms a three-dimensional reticular structure, increases the toughness and the high temperature resistance of the epoxy resin, can be cured at 23 ℃ for 120 min, can resist 350 ℃ for a long time, resist 450 ℃ for an instant time, has good elasticity and high-temperature sealing performance, has high electrical insulation performance and good fatigue resistance, can be used for plane sealing and caulking under high-temperature working conditions, particularly for repairing in a drying cylinder, has strong adhesion with temperature resistance of more than 280 ℃, has certain toughness after curing, and can adapt to thermal expansion and cold contraction of the drying cylinder under different temperatures.
The above description is only for the preferred embodiment of the present invention, but the scope of the present invention is not limited thereto, and any changes or substitutions that can be easily conceived by those skilled in the art within the technical scope of the present invention are also included in the scope of the present invention. Therefore, the protection scope of the present invention shall be subject to the protection scope of the claims.

Claims (10)

1. The special high-temperature repairing agent for dryer leakage stoppage is characterized by comprising the following components in parts by mass of 35-70:5-10: 1-20: 2-25.
2. The special high-temperature repairing agent for dryer leak stoppage according to claim 1, wherein the polyorganosiloxane is one or more of polydimethylsiloxane, hydroxyl-terminated linear polydimethylsiloxane, cyclic polydimethylsiloxane and divinyl polydimethylsiloxane.
3. The special high-temperature repairing agent for leaking stoppage of the drying cylinder as claimed in claim 1, wherein the white carbon black is hydrophobic white carbon black.
4. The special high-temperature repairing agent for dryer leaking stoppage according to claim 1, wherein the filler is inorganic non-metal particles and/or organic filler, the inorganic non-metal particles are one or more of nano silicon carbide, nano calcium carbonate, talcum powder, nano aluminum oxide, nano titanium oxide, kaolin and mica powder, the inorganic non-metal particles further comprise hydrophobic surface treatment particles, and the organic filler is one or more of styrene acrylonitrile copolymer particles, acrylonitrile-butadiene-styrene copolymer particles and polyvinyl butyral powder.
5. The special high-temperature repairing agent for leaking stoppage of the drying cylinder as claimed in claim 1, wherein the high-temperature epoxy resin is glycidyl ether epoxy resin, thermoplastic resin, diamine and solvent in a mass ratio of 50-65: 5-15: 4-8: 10-20.
6. The special high-temperature repairing agent for dryer leak stoppage according to claim 5, wherein the glycidyl ether type epoxy resin is one or more of bisphenol A type epoxy resin, phenol formaldehyde type epoxy resin, o-benzaldehyde type epoxy resin, resorcinol formaldehyde type epoxy resin, tris (hydroxyphenyl) methane type epoxy resin and polyol glycidyl ether type epoxy resin, the thermoplastic resin is one or more of bismaleimide resin BMI, polyimide resin PI and polyetherimide PEI, the diamine is one or more of diaminodiphenylmethane DDM, diaminodiphenyl ether DDE and diaminodiphenyl sulfone DDS, and the solvent is acetone, methanol or xylene.
7. The special high-temperature repairing agent for leaking stoppage of the drying cylinder as claimed in claim 1, wherein when the high-temperature repairing agent is used for repairing defects in the drying cylinder, construction is carried out at the temperature of more than or equal to 15 ℃ and the humidity of less than or equal to 90%, the rust remover is adopted for treating and cooling an oxide layer of the cylinder body and the cylinder cover, grinding a joint part of the cylinder body and the cylinder cover, uniformly coating the high-temperature repairing agent on the defects, pressurizing and compacting after curing, secondarily coating the high-temperature repairing agent, and curing for 8-12 hours.
8. The preparation method of the special high-temperature repairing agent for dryer leaking stoppage according to any one of claims 1 to 7, which is characterized by comprising the following steps: taking polyorganosiloxane into white carbon black and filler, shearing at the speed of 600 plus 1000rpm for 20-40min, adding high-temperature epoxy resin according to the random mixing principle, and uniformly stirring to prepare the high-temperature repairing agent, wherein the mass ratio of the polyorganosiloxane to the white carbon black to the filler to the high-temperature epoxy resin is 35-70:5-10: 1-20: 2-25.
9. The preparation method of the special high-temperature repairing agent for dryer leaking stoppage according to claim 8, wherein the white carbon black/filler is subjected to hydrophobic surface treatment, and the treatment steps are as follows: taking precipitated silica/filler and water, stirring for 5-10min, adding a silane coupling agent, dissolving in a solvent, stirring for 10-30min, aging for 1-2h, filtering, taking a filter cake, washing and drying with ethanol to obtain hydrophobic silica/hydrophobic surface filler, wherein the mass ratio of the precipitated silica/filler, water, the silane coupling agent and the solvent is 80-90: 100-150:2-4:12-30, wherein the silane coupling agent is one or more of KH560, KH792 and DL602, and the solvent is acetone, methanol or benzene.
10. The preparation method of the special high-temperature repairing agent for dryer plugging as claimed in claim 8, wherein the high-temperature epoxy resin is prepared by sequentially adding the thermoplastic resin and the diamine after the glycidyl ether epoxy resin and the solvent are stirred and preheated, and stirring for 20-30min at 60-75 ℃ and 200-400 rpm.
CN202111061368.5A 2021-09-10 2021-09-10 Special high-temperature repairing agent for leaking stoppage of drying cylinder Pending CN113621341A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN202111061368.5A CN113621341A (en) 2021-09-10 2021-09-10 Special high-temperature repairing agent for leaking stoppage of drying cylinder

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CN202111061368.5A CN113621341A (en) 2021-09-10 2021-09-10 Special high-temperature repairing agent for leaking stoppage of drying cylinder

Publications (1)

Publication Number Publication Date
CN113621341A true CN113621341A (en) 2021-11-09

Family

ID=78389760

Family Applications (1)

Application Number Title Priority Date Filing Date
CN202111061368.5A Pending CN113621341A (en) 2021-09-10 2021-09-10 Special high-temperature repairing agent for leaking stoppage of drying cylinder

Country Status (1)

Country Link
CN (1) CN113621341A (en)

Citations (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN101939396A (en) * 2007-09-19 2011-01-05 东丽株式会社 Adhesive composition for electronic parts and adhesive sheet for electronic parts using the same
CN102816552A (en) * 2011-06-08 2012-12-12 苏州达同新材料有限公司 Organosilicon encapsulating adhesive used for electrical and electronic products, and preparation method thereof
CN103242790A (en) * 2013-05-15 2013-08-14 东华大学 High temperature resistant mica tape adhesive and preparation method thereof
CN104804692A (en) * 2015-05-05 2015-07-29 南京信息工程大学 Double-component aluminum metal anti-corrosion repairing agent and preparation method thereof
CN105440998A (en) * 2015-11-26 2016-03-30 河南豫冠化工科技开发有限公司 Low-temperature fast-curing epoxy resin adhesive and preparation method thereof

Patent Citations (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN101939396A (en) * 2007-09-19 2011-01-05 东丽株式会社 Adhesive composition for electronic parts and adhesive sheet for electronic parts using the same
CN102816552A (en) * 2011-06-08 2012-12-12 苏州达同新材料有限公司 Organosilicon encapsulating adhesive used for electrical and electronic products, and preparation method thereof
CN103242790A (en) * 2013-05-15 2013-08-14 东华大学 High temperature resistant mica tape adhesive and preparation method thereof
CN104804692A (en) * 2015-05-05 2015-07-29 南京信息工程大学 Double-component aluminum metal anti-corrosion repairing agent and preparation method thereof
CN105440998A (en) * 2015-11-26 2016-03-30 河南豫冠化工科技开发有限公司 Low-temperature fast-curing epoxy resin adhesive and preparation method thereof

Non-Patent Citations (3)

* Cited by examiner, † Cited by third party
Title
孙曼灵等: "《环氧树脂应用原理与技术》", 30 September 2002, 机械工业出版社 *
张宪荣等: "《现代设计辞典》", 30 December 1998, 北京理工大学出版社 *
杨世英等: "《工程塑料手册》", 31 August 1994, 中国纺织出版社 *

Similar Documents

Publication Publication Date Title
CN110484025B (en) Method for improving settling resistance and dispersibility of silicon micro powder in organic silicon pouring sealant
CN110903608A (en) High-thermal-conductivity epoxy composite material and preparation method thereof
CN104910632A (en) Low-temperature vulcanized heat-conducting silicone rubber and preparation method thereof
CN112374798B (en) Preparation method of wear-resistant and impact-resistant epoxy mortar repair material
CN112143301B (en) Thermosetting corrosion-resistant wear-resistant coating material and preparation and use methods thereof
CN106433034A (en) Method for preparing amino functionalized carbon nanotube/epoxy resin compound material
Yu et al. Influence of nano-AlN particles on thermal conductivity, thermal stability and cure behavior of cycloaliphatic epoxy/trimethacrylate system.
CN111548760A (en) Epoxy resin adhesive and preparation method thereof
CN115746404B (en) Surface modified hexagonal boron nitride nanosheet, modification method thereof and epoxy composite material
Chen et al. Thermally conductive, healable glass fiber cloth reinforced polymer composite based on β-hydroxyester bonds crosslinked epoxy with improved heat resistance
CN113185915A (en) Preparation method of high-temperature-resistant organic silicon resin coating
CN115975526A (en) A kind of low hygroscopic epoxy adhesive film and preparation method thereof
CN103881379B (en) Hydroxy silicate/phosphorous benzoxazine/bismaleimide resin composite material and preparation method thereof
CN113621341A (en) Special high-temperature repairing agent for leaking stoppage of drying cylinder
Jiang et al. Effects of different nano‐SiO2/silane coupling agent “rigid‐flexible” hybrid interfaces on the mechanical performance of basalt fiber/epoxy composites
CN110628183B (en) A kind of epoxy glass fiber nanocomposite material for high-voltage switch insulating pull rod and preparation method thereof
CN116162328B (en) Liquid rubber and modified carbon black synergistically toughened epoxy resin and preparation method thereof
CN116715878B (en) An efficient preparation method for high temperature resistant and wave-transmitting micro-nano multi-scale quartz fiber cloth reinforced thermoplastic composite material
CN110628170B (en) A kind of graphene oxide-phenolic aerogel material based on silane modification and preparation method thereof
CN116239334A (en) Disk brake pad friction material and production process thereof
CN117624833A (en) Preparation method for improving thermal conductivity of epoxy resin based on core-shell structure
CN102153836B (en) Ionic liquid layered silicate/epoxide resin nano composite material and preparation method of ionic liquid layered silicate/epoxide resin nano composite material
CN117165152B (en) Preparation method of high surface tension NdFeB magnet anticorrosion coating
CN116355407B (en) Integrated preparation method of nano-alumina modified polyimide composite material
Xu et al. Improving thermal stability and mechanical properties of high temperature carbon fibre phthalonitrile resin composites via Nano-CuO modified matrices

Legal Events

Date Code Title Description
PB01 Publication
PB01 Publication
SE01 Entry into force of request for substantive examination
SE01 Entry into force of request for substantive examination