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GB2219802A - Bitumen composition - Google Patents

Bitumen composition Download PDF

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Publication number
GB2219802A
GB2219802A GB8814467A GB8814467A GB2219802A GB 2219802 A GB2219802 A GB 2219802A GB 8814467 A GB8814467 A GB 8814467A GB 8814467 A GB8814467 A GB 8814467A GB 2219802 A GB2219802 A GB 2219802A
Authority
GB
United Kingdom
Prior art keywords
bitumen
blend
polyethylene
softening point
roofing
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Withdrawn
Application number
GB8814467A
Other versions
GB8814467D0 (en
Inventor
Andrew Thompson
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
VULCANITE Ltd
Original Assignee
VULCANITE Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by VULCANITE Ltd filed Critical VULCANITE Ltd
Priority to GB8814467A priority Critical patent/GB2219802A/en
Publication of GB8814467D0 publication Critical patent/GB8814467D0/en
Priority to GB8913954A priority patent/GB2223229B/en
Publication of GB2219802A publication Critical patent/GB2219802A/en
Withdrawn legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L95/00Compositions of bituminous materials, e.g. asphalt, tar, pitch
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N5/00Roofing materials comprising a fibrous web coated with bitumen or another polymer, e.g. pitch
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N7/00Flexible sheet materials not otherwise provided for, e.g. textile threads, filaments, yarns or tow, glued on macromolecular material
    • D06N7/0063Floor covering on textile basis comprising a fibrous top layer being coated at the back with at least one polymer layer, e.g. carpets, rugs, synthetic turf
    • D06N7/0071Floor covering on textile basis comprising a fibrous top layer being coated at the back with at least one polymer layer, e.g. carpets, rugs, synthetic turf characterised by their backing, e.g. pre-coat, back coating, secondary backing, cushion backing
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N2203/00Macromolecular materials of the coating layers
    • D06N2203/04Macromolecular compounds obtained by reactions only involving carbon-to-carbon unsaturated bonds
    • D06N2203/042Polyolefin (co)polymers
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N2203/00Macromolecular materials of the coating layers
    • D06N2203/08Bituminous material, e.g. asphalt, tar, bitumen
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N2207/00Treatments by energy or chemical effects
    • D06N2207/08Treatments by energy or chemical effects using gas
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N2209/00Properties of the materials
    • D06N2209/12Permeability or impermeability properties
    • D06N2209/126Permeability to liquids, absorption
    • D06N2209/128Non-permeable
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06NWALL, FLOOR, OR LIKE COVERING MATERIALS, e.g. LINOLEUM, OILCLOTH, ARTIFICIAL LEATHER, ROOFING FELT, CONSISTING OF A FIBROUS WEB COATED WITH A LAYER OF MACROMOLECULAR MATERIAL; FLEXIBLE SHEET MATERIAL NOT OTHERWISE PROVIDED FOR
    • D06N2209/00Properties of the materials
    • D06N2209/16Properties of the materials having other properties
    • D06N2209/1692Weather resistance

Landscapes

  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Textile Engineering (AREA)
  • Civil Engineering (AREA)
  • Materials Engineering (AREA)
  • Structural Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Compositions Of Macromolecular Compounds (AREA)

Abstract

A bitumen blend comprises bitumen and a polymer binder, which is low density polyethylene most preferably having a melt flow index of from 0.3 to 0.4 and which most preferably also, is present from about 15 to 18% by weight. The softening point of the blend is preferably about 107 to 120 DEG C. The composition may be used as a waterproofing compound for roofing or for use in carpet tile backings.

Description

BITUMENlPOLYETHYLENE BLEND FOR ROOFING AND THE LIKE This invention relates to a modified bitumen blend for use particularly but not exclusively in roofing.
Roofing may be waterproofed by the application of a coated bituminous membrane or laminate. Conventionally, such felt has comprised of a layer of rag base - fibreglass, paper or hessian coated with oxidised bitumen and bonded by hot oxidised bitumen.
Bitumen may be oxidised to improve its mechanical properties, but other developments, as described in U,S. Patent No. 4368228, include modifying the bitumen with polymers such as styrene-butadiene-styrene block copolymer, atactic polypropylene, and polyisobutylene.
The examples in the patent show a polypropylene blend further modified by amorphous ethylenejpropylene copolymer.
A desirable bitumen blend should have a good processing viscosity at the coating temperature, a high softening point to resist slump in summer and good low temperature flexibility to prevent cracking in winter it is very desirable that the rheological changes described be achieved with a minimum addition of modifying compound.
It is an object of the present invention to provide a useable bitumen for roofing and the like, by an addition of at least 12% by weight of a modifying compound.
According to the present invention there is provided a bitumen blend for roofing damp courses and carpet tile backings, comprising bitumen and at least 12% by weight of a low density polyethylene (hereinafter polyethylene) having a melt flow index of from 0.2 to 005.
Preferably the melt flow index is 0.3 to 0.4 and more preferably there is from 15 to 18% by weight polyethylene.
In the production of, for example, the roofing felt ar.d the base materials used are standard and form no part of the invention.
As shown in Graph 1, for a bitumen/polyethlene blend, the softening point increases sharply past a critical concentration of modifying polymer, possibly as a polymer network is formed (see upper plateau in Graph 1). The inventor has however, found that a surprisingly low concentration of polyethylene is actually required to form a continuous phase of polyethylene, with a good processing viscosity. As can be seen from the aforementioned U.S. Patent, the trend is towards highly amorphous systems, with the minimum concentration of modifying polymer.It is therefore highly surprising.on a hindsight comparison with the apparently more amorphous atactic polypropylene (at least 20% by weight)- that the inventor has found a cost effective bitumen blend which requires only at least 12% by weight of a polyethylene, the characteristics of which are hereinbefore defined.
The bitumen/polyethylene blend can be used in (for example) the production of roofing materials dampcourse and in carpet tile backings The blend is prepared by mixing straight run bitumen, preferably 200pen, (BS4691) with low density polyethylene of melt flow index 0.2 to 0.5 preferably 0.3 to 0.4 where the polyethylene may vary from about 12% to 20%, at an elevated temperature, until a smooth dispersion mixture, with a softening point in the region of 107degC-120degC, is obtained.This mixture may be filled with a mineral filler such as calcium carbonate, fly ash or slate dust, up to a loading of 40% Once the mixture has been prepared, it may be applied using conventional techniques to rag fibre, paper, fibreglass, asbestos, hessian and polyester bases, or any combination of the aforementioned in a laminate, to produce a water-proofing membrane which may be finished with sand, talc, slate granules or aluminium flakes on the top surface and, in the case of traditional roll and ppur felts, sand on the bottom or with a cast polypropylene/ polyethylene film where the product is to be applied with a gas torch.
The invention will now be described by way of example: Exaluple 1 The composition of a typical mixture which may be advantageously used in the manner described above would be:200 pen bitumen - 86%) 60% low density polyethylene(BS3412) - 14%) limestone filler 40,0 This mixture would also be suitable for carpet tile backing in place of conventional filled oxidised bitumen.
The advantage of polyethylene midified bitumen over conventional oxidised bitumen are:1. Improved resistance against slump at high temperatures.
2. Improved low temperatux flexibility (down to -lOdegC).
3. Improved ductility.
Example 2 The following blend was prepared again as before:15% polyethylene ! 70% 85t 200pen ) Filler 30% Four tests were carried out on this blend to determine its suitability: the softening point, penetration at 250C, the low temperature flex and the viscosity at typical processing temperatures. The softening point must be high enough to avoid substantial slump in the summer yet have sufficient flexibility to avoid brittleness in the winter.
The blend should further have reasonable hardness and a reasonable processing viscosity.
The following properties noted, and a graph (No. 2) prepared of viscosity against temperature for example 2: a. softening point - llldegC b. penetration @ 25degC - 23dmm c. low temperature flex - lOdegC D. viscosities at 155 degC - 11900 cps " " 160degC - 9300 cps " " 165degC - 7900 cps It It l70degC - 6700 cps Results were tabulated (table 1) showing the temperature.jviscosity characteristics of bitumen blend, at specific percentages of polyethylene.
Bitumen/P.E. blends Results 3% P.E. SP - 62"0 Temp viscosity (cp) 140 800 150 600 160 400 170 350 180 300 6% P.E. SP - 74 C Temp viscosity (cp) 140 3,200 150 2,400 160 1,700 170 1,300 180 1,100 9% P.E. SP - 1000C Temp Viscosity 140 3,800 150 3,300 160 2,700 170 2,000 180 1,500 12% P.E. SP - 107"0 Temp Viscosity 140 20,200 150 12,300 160 7,900 170 6,400 180 4,900 As shown in Table 1 and graph 1, there is a sharp rise in the viscosity and softening point of the bitumen blend surprisingly between about 6% and J2% of polyethylene addition.Thereafter the softening point increases only slightly with further addition of polyethylene.Thus below about 6% ptlyethylene there is a dispersion of polyethylene in a continuous bitumen phase; from about 6% to about 12%, there is phase inversion; and about 12% and above the polyethylene in the continuous phase. Above about 20% the blend becomes too viscous for piratical use. The inventor has therefore found that an apparently less amorphous system in comparative terms actually requires a good deal less modifying polymer to bring about phase inversion, than say bitumen/polypropylene, and have thereby found a useable and cost effective bitumen blend.
Furthermore, as can be seen from the rest of the results of example 2 and the graphs, the softening point, low temperature flex and penetration are superior to conventional oxidised bitumen (95/25; 111/15) presently being used by the roofing industry. The viscosity is good for processing of the blend, intact at the normal processing temperature of about 1600C, the resulting viscosity of 9300cps was ideal-and the blend can be surprisingly produced at a cost effective minimum addition of about 12% of the defined polyethylene.
It will be appreciated that further polymers such as selectively shown from the aforementioned U.S. Patent can be added to further modify the bitumen/polyethylene blend.

Claims (5)

CLAIMS:
1. A bitumen blend for roofing damp courses and carpet tile backings, comprising bitumen and at least 12% by weight ofa low density polyethylene having a melt flow index of from 0.2 to 0.5.
2. A bitumen blend as claimed in claim 1 wherein the melt flow index of the low density polyethylene is from 0.3 to 0.4.
3 A bitumen blend as claimed in claims 1 and 2 wherein there is from 15 to 18% by weight low density polyethylene present.
4. A bitumen blend as claimed in any one of claims 1 to 3, which has a softening point of about 107 to 1200C.
5. A bitumen blend substantially as described herein with particular. reference to the examples.
GB8814467A 1988-06-17 1988-06-17 Bitumen composition Withdrawn GB2219802A (en)

Priority Applications (2)

Application Number Priority Date Filing Date Title
GB8814467A GB2219802A (en) 1988-06-17 1988-06-17 Bitumen composition
GB8913954A GB2223229B (en) 1988-06-17 1989-06-16 Modified bitumen blend for roofing and the like

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
GB8814467A GB2219802A (en) 1988-06-17 1988-06-17 Bitumen composition

Publications (2)

Publication Number Publication Date
GB8814467D0 GB8814467D0 (en) 1988-07-20
GB2219802A true GB2219802A (en) 1989-12-20

Family

ID=10638898

Family Applications (2)

Application Number Title Priority Date Filing Date
GB8814467A Withdrawn GB2219802A (en) 1988-06-17 1988-06-17 Bitumen composition
GB8913954A Expired - Lifetime GB2223229B (en) 1988-06-17 1989-06-16 Modified bitumen blend for roofing and the like

Family Applications After (1)

Application Number Title Priority Date Filing Date
GB8913954A Expired - Lifetime GB2223229B (en) 1988-06-17 1989-06-16 Modified bitumen blend for roofing and the like

Country Status (1)

Country Link
GB (2) GB2219802A (en)

Cited By (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO1991015625A1 (en) * 1990-04-10 1991-10-17 Interface, Inc. Floor covering with bitumen backing layer
EP0500379A1 (en) * 1991-02-22 1992-08-26 Milliken Research Corporation Bitumen backed carpet tile
EP0622422A1 (en) * 1993-04-29 1994-11-02 Exxon Chemical Patents Inc. Compositions for construction materials
US5366779A (en) * 1990-04-10 1994-11-22 Interface, Inc. Floor covering with bitumen backing layer
US5380773A (en) * 1991-12-23 1995-01-10 Ecp Enichem Polimeri S.R.L. Bitumens modified with recycled and/or virgin polymers and their applications
EP1247891A3 (en) * 2001-04-05 2004-05-06 Collins & Aikman Floorcoverings, Inc. A carpet tile containing resin and bitumen processed at low temperatures
US7317045B2 (en) 2005-09-06 2008-01-08 Natalino Zanchetta Polyethylene modified asphalt compositions

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO1996005716A2 (en) * 1994-08-18 1996-02-29 Anatoly Alexeevich Bespalov Method of removing crude oil or oil products from a surface, a method of regenerating and a method of using the used product
ES2136532B1 (en) * 1997-01-31 2000-07-01 Repsol Petroleo Sa BETUNES MODIFIED WITH POLYETHYLENE FOR IMPROVED COMPATIBILITY.

Citations (13)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB1238365A (en) * 1967-11-11 1971-07-07
GB1348385A (en) * 1970-05-05 1974-03-13 Nynaes Petroleum Ab Corrugated board and a method for its manufacture
GB1408865A (en) * 1971-09-07 1975-10-08 Haberl P Process for the production of a mixture containing bitumen
GB1417571A (en) * 1972-02-11 1975-12-10 Ruberoid Ltd Self-adhesive bituminous composition
GB1509943A (en) * 1974-08-28 1978-05-10 Basf Ag Mixtures based on ethylene copolymers and bitumen
GB1519508A (en) * 1974-10-19 1978-07-26 Huels Chemische Werke Ag Process for the manufacture of homogeneous thermoplastic compositions in the form of ribbon or granules
GB1521694A (en) * 1974-09-13 1978-08-16 Bunzl & Biach Ag Method of preparing a bituminous binder and a construction material containing the same
EP0009432A1 (en) * 1978-09-13 1980-04-02 COMPOSANTS INDUSTRIALISES DU BATIMENT par abréviation C.I.B. Société dite: Bituminous compositions containing polymers and their applications
SU808440A1 (en) * 1979-03-11 1981-02-28 Белорусский Ордена Трудовогокрасного Знамени Политехническийинститут Bituminous mineral mixture
SU885497A1 (en) * 1980-01-21 1981-11-30 Всесоюзный научно-исследовательский и проектно-конструкторский институт кровельных и гидроизоляционных материалов и изделий Hydro-insulating composition
SU920163A1 (en) * 1980-03-21 1982-04-15 Всесоюзный научно-исследовательский и проектно-конструкторский институт кровельных и гидроизоляционных материалов и изделий Hydralic insulation composition
EP0131397A1 (en) * 1983-06-28 1985-01-16 Exxon Research And Engineering Company Bitumenous compositions
DE3601371A1 (en) * 1986-01-18 1987-07-23 Ruetgerswerke Ag Support sheet for shingles

Family Cites Families (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
IT1223336B (en) * 1987-11-02 1990-09-19 Enichem Anic Spa BITUMINOUS COMPOSITION AND ITS USE IN THE WATERPROOFING SECTOR

Patent Citations (13)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB1238365A (en) * 1967-11-11 1971-07-07
GB1348385A (en) * 1970-05-05 1974-03-13 Nynaes Petroleum Ab Corrugated board and a method for its manufacture
GB1408865A (en) * 1971-09-07 1975-10-08 Haberl P Process for the production of a mixture containing bitumen
GB1417571A (en) * 1972-02-11 1975-12-10 Ruberoid Ltd Self-adhesive bituminous composition
GB1509943A (en) * 1974-08-28 1978-05-10 Basf Ag Mixtures based on ethylene copolymers and bitumen
GB1521694A (en) * 1974-09-13 1978-08-16 Bunzl & Biach Ag Method of preparing a bituminous binder and a construction material containing the same
GB1519508A (en) * 1974-10-19 1978-07-26 Huels Chemische Werke Ag Process for the manufacture of homogeneous thermoplastic compositions in the form of ribbon or granules
EP0009432A1 (en) * 1978-09-13 1980-04-02 COMPOSANTS INDUSTRIALISES DU BATIMENT par abréviation C.I.B. Société dite: Bituminous compositions containing polymers and their applications
SU808440A1 (en) * 1979-03-11 1981-02-28 Белорусский Ордена Трудовогокрасного Знамени Политехническийинститут Bituminous mineral mixture
SU885497A1 (en) * 1980-01-21 1981-11-30 Всесоюзный научно-исследовательский и проектно-конструкторский институт кровельных и гидроизоляционных материалов и изделий Hydro-insulating composition
SU920163A1 (en) * 1980-03-21 1982-04-15 Всесоюзный научно-исследовательский и проектно-конструкторский институт кровельных и гидроизоляционных материалов и изделий Hydralic insulation composition
EP0131397A1 (en) * 1983-06-28 1985-01-16 Exxon Research And Engineering Company Bitumenous compositions
DE3601371A1 (en) * 1986-01-18 1987-07-23 Ruetgerswerke Ag Support sheet for shingles

Cited By (10)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO1991015625A1 (en) * 1990-04-10 1991-10-17 Interface, Inc. Floor covering with bitumen backing layer
AU646041B2 (en) * 1990-04-10 1994-02-03 Interface, Inc. Floor covering with bitumen backing layer
US5366779A (en) * 1990-04-10 1994-11-22 Interface, Inc. Floor covering with bitumen backing layer
EP0500379A1 (en) * 1991-02-22 1992-08-26 Milliken Research Corporation Bitumen backed carpet tile
AU651172B2 (en) * 1991-02-22 1994-07-14 Milliken Research Corporation Bitumen backed carpet tile
US5929145A (en) * 1991-02-22 1999-07-27 Milliken & Company Bitumen backed carpet tile
US5380773A (en) * 1991-12-23 1995-01-10 Ecp Enichem Polimeri S.R.L. Bitumens modified with recycled and/or virgin polymers and their applications
EP0622422A1 (en) * 1993-04-29 1994-11-02 Exxon Chemical Patents Inc. Compositions for construction materials
EP1247891A3 (en) * 2001-04-05 2004-05-06 Collins & Aikman Floorcoverings, Inc. A carpet tile containing resin and bitumen processed at low temperatures
US7317045B2 (en) 2005-09-06 2008-01-08 Natalino Zanchetta Polyethylene modified asphalt compositions

Also Published As

Publication number Publication date
GB8814467D0 (en) 1988-07-20
GB2223229A (en) 1990-04-04
GB2223229B (en) 1991-10-09
GB8913954D0 (en) 1989-08-02

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