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ITMI20110227A1 - COMPOSITE LAMINATE IN PARTICULAR FOR NAUTICAL APPLICATIONS AND RELATIVE MANUFACTURING PROCESS - Google Patents

COMPOSITE LAMINATE IN PARTICULAR FOR NAUTICAL APPLICATIONS AND RELATIVE MANUFACTURING PROCESS Download PDF

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Publication number
ITMI20110227A1
ITMI20110227A1 IT000227A ITMI20110227A ITMI20110227A1 IT MI20110227 A1 ITMI20110227 A1 IT MI20110227A1 IT 000227 A IT000227 A IT 000227A IT MI20110227 A ITMI20110227 A IT MI20110227A IT MI20110227 A1 ITMI20110227 A1 IT MI20110227A1
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IT
Italy
Prior art keywords
resins
laminate according
weight
fabric
finished product
Prior art date
Application number
IT000227A
Other languages
Italian (it)
Inventor
Maurizio Marcassoli
Original Assignee
Filp S P A
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Filp S P A filed Critical Filp S P A
Priority to ITMI2011A000227A priority Critical patent/IT1403939B1/en
Publication of ITMI20110227A1 publication Critical patent/ITMI20110227A1/en
Application granted granted Critical
Publication of IT1403939B1 publication Critical patent/IT1403939B1/en

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Classifications

    • BPERFORMING OPERATIONS; TRANSPORTING
    • B32LAYERED PRODUCTS
    • B32BLAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B27/00Layered products comprising a layer of synthetic resin
    • B32B27/42Layered products comprising a layer of synthetic resin comprising condensation resins of aldehydes, e.g. with phenols, ureas or melamines
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B32LAYERED PRODUCTS
    • B32BLAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B27/00Layered products comprising a layer of synthetic resin
    • B32B27/04Layered products comprising a layer of synthetic resin as impregnant, bonding, or embedding substance
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B32LAYERED PRODUCTS
    • B32BLAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B5/00Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts
    • B32B5/22Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed
    • B32B5/24Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed one layer being a fibrous or filamentary layer
    • B32B5/26Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed one layer being a fibrous or filamentary layer another layer next to it also being fibrous or filamentary
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B32LAYERED PRODUCTS
    • B32BLAYERED PRODUCTS, i.e. PRODUCTS BUILT-UP OF STRATA OF FLAT OR NON-FLAT, e.g. CELLULAR OR HONEYCOMB, FORM
    • B32B5/00Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts
    • B32B5/22Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed
    • B32B5/24Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed one layer being a fibrous or filamentary layer
    • B32B5/28Layered products characterised by the non- homogeneity or physical structure, i.e. comprising a fibrous, filamentary, particulate or foam layer; Layered products characterised by having a layer differing constitutionally or physically in different parts characterised by the presence of two or more layers which are next to each other and are fibrous, filamentary, formed of particles or foamed one layer being a fibrous or filamentary layer impregnated with or embedded in a plastic substance

Landscapes

  • Laminated Bodies (AREA)

Description

DESCRIZIONE DESCRIPTION

La presente invenzione riguarda un laminato composito, in particolare per applicazioni nautiche. The present invention relates to a composite laminate, in particular for nautical applications.

Laminati compositi, realizzati a partire da più strati di tessuti di fibra, per lo più fibra naturale, impregnati di resina termoindurente e fatti indurire in modo opportuno, trovano diversi campi di applicazione data la loro elevata resistenza meccanica e inalterabilità all’invecchiamento, anche in seguito ad esposizione a condizioni ambientali severe, come umidità, esposizione solare, temperature elevate e anche salsedine. Composite laminates, made from several layers of fiber fabrics, mostly natural fiber, impregnated with thermosetting resin and hardened appropriately, find different fields of application given their high mechanical resistance and inalterability to aging, even following exposure to severe environmental conditions, such as humidity, sun exposure, high temperatures and even saltiness.

I laminati possono, a seconda dello spessore, comprendere decine o centinaia di strati di tessuto sovrapposti. Gli strati vengono impregnati con la resina, miscelata ad una opportuna quantità di solvente di tipo adatto per conferire adeguate proprietà reologiche, e posti in una pressa a caldo, a temperatura in genere sui 130°C e pressioni intorno ai 150 Kgf/cm<2>. L’indurimento avviene grazie alla reazione di policondensazione ed il solvente evapora. The laminates can, depending on the thickness, comprise tens or hundreds of overlapping fabric layers. The layers are impregnated with the resin, mixed with an appropriate quantity of solvent of a suitable type to give adequate rheological properties, and placed in a hot press, at a temperature generally around 130 ° C and pressures around 150 Kgf / cm <2 >. The hardening takes place thanks to the polycondensation reaction and the solvent evaporates.

Un particolare campo di applicazione à ̈ quello nautico. Per esempio, laminati di questo tipo sono impiegati nella realizzazione di coperte di natanti, come barche o battelli, in sostituzione del legno, in particolare in sostituzione di legni pregiati, come il mogano e il teak. Infatti alla resistenza meccanica, in particolare resistenza a flessione, all’impatto, la lavorabilità, compresa la possibilità di procedere a carteggiatura o simili operazioni, lavorabilità paragonabile a quella del legno tali laminati uniscono caratteristiche che le rendono anche superiore al legno in termini di prestazioni. In particolare l’indeformabilità, tale da rendere superflue operazioni di calatafaggio e la durata, nelle condizioni severe tipiche di un ambiente marino, molto superiore al legno. Inoltre i laminati, anche grazie al tessuto, hanno una superficie non scivolosa, all’occhio ed al tatto simile al legno, che non si scalda più del legno all’esposizione al sole ed à ̈ verniciabile, anche con comuni impregnanti ad olio. A particular field of application is the nautical one. For example, laminates of this type are used in the construction of decks for boats, such as boats or boats, to replace wood, in particular to replace precious woods, such as mahogany and teak. In fact, to the mechanical resistance, in particular resistance to bending, to impact, workability, including the possibility of sanding or similar operations, workability comparable to that of wood, these laminates combine characteristics that make them even superior to wood in terms of performance. In particular, the non-deformability, such as to make caulking operations unnecessary and the duration, in the severe conditions typical of a marine environment, much superior to wood. Furthermore, the laminates, also thanks to the fabric, have a non-slippery surface, to the eye and to the touch similar to wood, which does not heat up any more than wood when exposed to the sun and can be painted, even with common oil impregnating agents. .

Infine, i laminati, che possono avere spessore variabile, sono resistenti a flessione, non necessitano di supporti particolari per l’installazione e si possono facilmente incollare con colle di comune impiego, senza necessità di preparazione o di applicazione di primer. Infine non producono schegge. Finally, the laminates, which can have variable thickness, are resistant to bending, do not require special supports for installation and can be easily glued with commonly used glues, without the need for preparation or application of primer. Finally, they do not produce splinters.

I laminati in resina a base fenolica o cresilica sono utilizzati perché possono avere un colore simile a quello dei legni più pregiati, che unito ad un aspetto della superficie simile al legno ne fanno ottimi sostituti, più economici e con prestazioni meccaniche e di resistenza superiori. Tuttavia, nonostante resistano all’esposizione solare per quanto riguarda resistenza ed indeformabilità, al pari del legno, i laminati tendono a subire alterazioni significative del colore, in particolare a scurire, nelle superfici esposte. Questo può rendere necessarie operazioni di carteggiatura o verniciatura, se si vuole ovviare a questo inconveniente. Anche l’aggiunta alla formulazione della resina dei comuni additivi anti UV, anche in forti quantità, oltre che ad aumentare il costo totale, dato il prezzo elevato di tali additivi, non permette di ottenere risultati soddisfacenti da questo punto di vista. Pertanto à ̈ desiderabile un laminato in resina a base fenolica o cresilica, avente le caratteristiche sopra esposte, e che risolva il problema della alterazione del colore in seguito ad esposizione solare. Il problema sopra esposto à ̈ ora stato risolto secondo la presente invenzione da un laminato composito termoindurente comprendente più strati di tessuto sovrapposti, per un 20-50% in peso, da 1 a 40%, preferibilmente dal 5 al 20% di una o più resine fenoliche o cresiliche o loro miscele, dal 10 al 60% di una o più resine melamminiche, preferibilmente dal 20 al 40%. Phenolic or cresyl-based resin laminates are used because they can have a color similar to that of the finest woods, which combined with a wood-like surface appearance make them excellent substitutes, cheaper and with superior mechanical and resistance performance. . However, despite being resistant to sunlight in terms of resistance and non-deformability, like wood, laminates tend to undergo significant color changes, in particular to darken, on exposed surfaces. This may make sanding or painting operations necessary if this problem is to be overcome. Even the addition of common anti UV additives to the resin formulation, even in large quantities, as well as increasing the total cost, given the high price of these additives, does not allow to obtain satisfactory results from this point of view. Therefore, a phenolic or cresyl-based resin laminate is desirable, having the characteristics described above, and which solves the problem of color alteration following sun exposure. The above problem has now been solved according to the present invention by a thermosetting composite laminate comprising several layers of superimposed fabric, for a 20-50% by weight, from 1 to 40%, preferably from 5 to 20% of one or more phenolic or cresyl resins or their mixtures, from 10 to 60% of one or more melamine resins, preferably from 20 to 40%.

Tutte le percentuali, salvo indicazione diversa, sono da intendersi in peso. All percentages, unless otherwise indicated, are by weight.

Preferibilmente il laminato comprende dal 10 all’80% di una o più resine epossidiche, più preferibilmente dal 15 al 30%. Preferably the laminate comprises from 10 to 80% of one or more epoxy resins, more preferably from 15 to 30%.

Secondo un ulteriore aspetto dell’invenzione, il laminato comprende uno o più additivi atti a conferire resistenza ai raggi UV, in percentuale dallo 0,01 allo 0,2%, in particolare un additivo del tipo con azoto eterociclico. According to a further aspect of the invention, the laminate comprises one or more additives suitable for conferring resistance to UV rays, in a percentage from 0.01 to 0.2%, in particular an additive of the type with heterocyclic nitrogen.

È stato trovato che la combinazione di resine sopra indicata conferisce al prodotto finale notevoli caratteristiche di resistenza alle alterazioni cromatiche dovute all’esposizione solare anche in presenza di piccole quantità di detti additivi, come sono quelle indicate sopra. It has been found that the combination of resins indicated above gives the final product remarkable characteristics of resistance to chromatic alterations due to sun exposure even in the presence of small quantities of said additives, such as those indicated above.

Il laminato secondo la presente invenzione può essere prodotto impregnando più strati sovrapposti di tessuto con una miscela di resine e di additivi, in quantità tali da rispettare le percentuali sopra indicate nel prodotto finito, disciolte in opportuno solvente, e sottoponendo il semilavorato ottenuto a pressatura a caldo, fino ad indurimento avvenuto. Il solvente, il tipo di tessuto, si intende che questo termine può comprendere anche tessuto non tessuto, anche se sono preferiti tessuti tessuti, in genere aventi una trama ed un ordito, possono essere del tipo usato nei laminati compositi dell’arte nota. Il solvente può, secondo una possibile forma di esecuzione, essere presente in quantità da costituire dal 10 al 30%, per esempio circa il 20%, del semilavorato impregnato, e può essere, per esempio, etanolo, acetone, metiletilchetone. The laminate according to the present invention can be produced by impregnating several superimposed layers of fabric with a mixture of resins and additives, in quantities such as to respect the percentages indicated above in the finished product, dissolved in a suitable solvent, and subjecting the semi-finished product obtained to pressing to hot, until hardening. The solvent, the type of fabric, it is understood that this term can also include non-woven fabric, even if woven fabrics are preferred, generally having a weft and a warp, they can be of the type used in the composite laminates of the known art. The solvent can, according to a possible embodiment, be present in quantities to constitute from 10 to 30%, for example about 20%, of the impregnated semi-finished product, and can be, for example, ethanol, acetone, methylethylketone.

Le resine sopra indicate, possono essere resine per impregnazione, comunemente presenti in commercio, per esempio commercializzate da Dow, SIR, Ciba o altri. The resins indicated above can be resins for impregnation, commonly present on the market, for example marketed by Dow, SIR, Ciba or others.

Gli additivi atti a conferire resistenza ai raggi UV sono di qualsiasi tipo adatto alle resine utilizzate, preferibilmente del tipo ad azoto eterociclico. The additives suitable for conferring resistance to UV rays are of any type suitable for the resins used, preferably of the heterocyclic nitrogen type.

I tessuti preferiti sono tessuti naturali, preferibilmente comprendenti fibre vegetali, per esempio canapa, juta, lino, cotone. The preferred fabrics are natural fabrics, preferably comprising vegetable fibers, for example hemp, jute, linen, cotton.

Per quanto riguarda la struttura e le modalità di realizzazione del laminato, eccetto che per la composizione di cui sopra, esse possono essere del tutto analoghe a quelle dei laminati dell’arte nota, in particolare quelli adatti ad applicazioni di tipo nautico. As regards the structure and methods of manufacturing the laminate, except for the above composition, they can be completely similar to those of the laminates of the known art, in particular those suitable for nautical applications.

È stato realizzato un laminato comprendente il 10% di una resina fenolica, il 29,95% di una resina melamminica, il 20% di una resina epossidica, il 40% di tessuto di cotone, disposto in strati sovrapposti e lo 0,05% di un additivo anti UV ad azoto eterociclico, con un processo secondo le modalità sopra indicate. A laminate was made comprising 10% of a phenolic resin, 29.95% of a melamine resin, 20% of an epoxy resin, 40% of cotton fabric, arranged in overlapping layers and 0.05% of an anti UV additive with heterocyclic nitrogen, with a process according to the methods indicated above.

Dopo prolungata esposizione a luce solare, per circa sei mesi in ambiente marino, tale da provocare un significativo scurimento dei laminati per applicazioni nautiche commercializzati da Filp SpA con la denominazione N-120 ed N-130 si à ̈ verificata una sostanziale assenza di alterazione del colore. After prolonged exposure to sunlight, for about six months in a marine environment, such as to cause a significant darkening of the laminates for nautical applications marketed by Filp SpA under the names N-120 and N-130, there was a substantial absence of alteration of the color.

Il confronto tra gli stessi laminati à ̈ anche stato fatto dopo esposizione per oltre 2000 h continuative ad un miscela di radiazioni simile a quello della naturale luce del sole, ottenuta con una lampada OSRAM ultra-vitalux 230v-E27-ES. The comparison between the same laminates was also made after exposure for over 2000 hours to a mixture of radiation similar to that of natural sunlight, obtained with an OSRAM ultra-vitalux 230v-E27-ES lamp.

Le caratteristiche meccaniche e di resistenza anche in particolari condizioni ambientali sono paragonabili a quelle di laminati per arte nota. La notevole resistenza all’alterazione del colore in seguito ad esposizione solare del laminato secondo la presente invenzione lo rendono particolarmente adatto ad applicazioni dove tale caratteristica sia vantaggiosa, come applicazioni nautiche, in particolare la costruzione delle coperte di natanti. The mechanical and resistance characteristics, even in particular environmental conditions, are comparable to those of laminates for the known art. The remarkable resistance to color alteration following sun exposure of the laminate according to the present invention makes it particularly suitable for applications where this characteristic is advantageous, such as nautical applications, in particular the construction of boat decks.

Claims (7)

RIVENDICAZIONI 1. Laminato composito termoindurente comprendente più strati di tessuto sovrapposti, per un 20-50%, da 1 a 40% di una o più resine fenoliche o cresiliche o loro miscele, dal 10 al 60% di una o più resine melamminiche, le percentuali essendo in peso. CLAIMS 1. Thermosetting composite laminate comprising several layers of superimposed fabric, for a 20-50%, from 1 to 40% of one or more phenolic or cresyl resins or their mixtures, from 10 to 60% of one or more melamine resins, the percentages being by weight. 2. Laminato secondo la rivendicazione 1 comprendente dal 10 all’ 80%, in particolare dal 15 al 30% in peso di una o più resine epossidiche. 2. Laminate according to claim 1 comprising from 10 to 80%, in particular from 15 to 30% by weight, of one or more epoxy resins. 3. Laminato secondo qualsiasi rivendicazione precedente, in cui le resine fenoliche o cresiliche sono presenti dal 5 al 20% in peso. 3. Laminate according to any preceding claim, wherein the phenolic or cresyl resins are present from 5 to 20% by weight. 4. Laminato secondo qualsiasi rivendicazione precedente, in cui le resine melamminiche sono presenti dal 20 al 40% in peso. 4. Laminate according to any preceding claim, wherein the melamine resins are present from 20 to 40% by weight. 5. Laminato secondo qualsiasi rivendicazione precedente, comprendente uno o più additivi atti a conferire resistenza ai raggi UV, in percentuale dallo 0,01 allo 0,2% in peso, in particolare un additivo del tipo con azoto eterociclico. 5. Laminate according to any preceding claim, comprising one or more additives suitable for conferring resistance to UV rays, in a percentage from 0.01 to 0.2% by weight, in particular an additive of the type with heterocyclic nitrogen. 6. Laminato secondo qualsiasi rivendicazione precedente, in cui il tessuto comprende fibra vegetale, in particolare cotone. 6. Laminate according to any preceding claim, wherein the fabric comprises vegetable fiber, in particular cotton. 7. Processo di fabbricazione di un laminato secondo qualsiasi rivendicazione precedente comprendente le seguenti fasi: impregnazione di più strati di tessuto con una miscela di resine ed additivi atti a conferire resistenza ai raggi UV in proporzioni tali da rispettare le percentuali nel prodotto finito ed un solvente adatto per ottenere un semilavorato impregnato; pressatura a caldo in condizioni opportune del semilavorato fino ad indurimento della miscela di resine ed evaporazione del solvente.7. Manufacturing process of a laminate according to any preceding claim comprising the following steps: impregnation of several layers of fabric with a mixture of resins and additives capable of conferring resistance to UV rays in proportions such as to respect the percentages in the finished product and a solvent suitable for obtaining an impregnated semi-finished product; hot pressing of the semi-finished product under suitable conditions until the resin mixture hardens and the solvent evaporates.
ITMI2011A000227A 2011-02-16 2011-02-16 COMPOSITE LAMINATE IN PARTICULAR FOR NAUTICAL APPLICATIONS AND RELATIVE MANUFACTURING PROCESS IT1403939B1 (en)

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ITMI2011A000227A IT1403939B1 (en) 2011-02-16 2011-02-16 COMPOSITE LAMINATE IN PARTICULAR FOR NAUTICAL APPLICATIONS AND RELATIVE MANUFACTURING PROCESS

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Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20070193683A1 (en) * 2006-02-17 2007-08-23 Halo Lsi, Inc. Continuous pressed laminates

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20070193683A1 (en) * 2006-02-17 2007-08-23 Halo Lsi, Inc. Continuous pressed laminates

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